Platform for the Accelerated Realization, Analysis, and Discovery of Interface Materials (PARADIM)

PARADIM helps users design and create new interface materials — materials that do not exist in nature — with unprecedented properties for the next generation of electronic devices. Creating new interface materials with unprecedented properties, by design rather than by serendipity, is accomplished in PARADIM through a synergistic set of user facilities dedicated to theory (figuring out where to put the atoms for useful behavior), synthesis (putting the atoms in the targeted positions), and characterization (seeing that the atoms are indeed in the desired positions).

Publications

  • C.  . Parzyck, A. Galdi, J.  . Nangoi, W.  .  . DeBenedetti, J. Balajka, B.  . Faeth, H. Paik, C. Hu, T.  . Arias, M.  . Hines, D.  . Schlom, K.  . Shen, and J.  . Maxson
    Single-Crystal Alkali Antimonide Photocathodes: High Efficiency in the Ultrathin Limit
    Physical Review Letters
    128
    (2022)
    10.1103/physrevlett.128.114801
  • J. N. Nelson, N. J. Schreiber, A. B. Georgescu, B. H. Goodge, B. D. Faeth, C. T. Parzyck, C. Zeledon, L. F. Kourkoutis, A. J. Millis, A. Georges, D. G. Schlom, and K. M. Shen
    Interfacial charge transfer and persistent metallicity of ultrathin SrIrO 3 /SrRuO 3 heterostructures
    Science Advances
    8
    (2022)
    10.1126/sciadv.abj0481
  • A. J. Mannix, A. Ye, S. H. Sung, A. Ray, F. Mujid, C. Park, M. Lee, J. Kang, R. Shreiner, A. A. High, D. A. Muller, R. Hovden, and J. Park
    Robotic four-dimensional pixel assembly of van der Waals solids
    Nature Nanotechnology
    17
    361-366
    (2022)
    10.1038/s41565-021-01061-5
  • S. H. Sung, N. Schnitzer, S. Novakov, I. El Baggari, X. Luo, J. Gim, N. M. Vu, Z. Li, T. H. Brintlinger, Y. Liu, W. Lu, Y. Sun, P. B. Deotare, K. Sun, L. Zhao, L. F. Kourkoutis, J. T. Heron, and R. Hovden
    Two-dimensional charge order stabilized in clean polytype heterostructures
    Nature Communications
    13
    (2022)
    10.1038/s41467-021-27947-5
  • T. Yu, J. Wright, G. Khalsa, B. Pamuk, C. S. Chang, Y. Matveyev, X. Wang, T. Schmitt, D. Feng, D. A. Muller, H. G. Xing, D. Jena, and V. N. Strocov
    Momentum-resolved electronic structure and band offsets in an epitaxial NbN/GaN superconductor/semiconductor heterojunction
    Science Advances
    7
    (2021)
    10.1126/sciadv.abi5833
  • Z. He, H. Guo, J. D. LaCoste, D. Werder, D. J. Durocher, R. A. Cook, P. Truong, H. Luo, X. Zhou, and L. Fei
    A Generalized Synthesis Strategy for Binderless, Free-Standing Anode for Lithium/Sodium Ion Battery Comprised of Metal Selenides@Carbon Nanofibers
    ACS Applied Energy Materials
    5
    842-851
    (2021)
    10.1021/acsaem.1c03277
  • G. A. Pan, D. Ferenc Segedin, H. LaBollita, Q. Song, E. M. Nica, B. H. Goodge, A. T. Pierce, S. Doyle, S. Novakov, D. Córdova Carrizales, A. T. N’Diaye, P. Shafer, H. Paik, J. T. Heron, J. A. Mason, A. Yacoby, L. F. Kourkoutis, O. Erten, C. M. Brooks, A. S. Botana, and J. A. Mundy
    Superconductivity in a quintuple-layer square-planar nickelate
    Nature Materials
    21
    160-164
    (2021)
    10.1038/s41563-021-01142-9
  • L. M. Garten, Z. Jiang, H. Paik, J. D. Perkins, A. Kakekhani, R. Fei, D. J. Werder, M. E. Holtz, D. S. Ginley, A. M. Rappe, D. G. Schlom, and M. L. Staruch
    Stromataxic Stabilization of a Metastable Layered ScFeO3 Polymorph
    Chemistry of Materials
    33
    7423-7431
    (2021)
    10.1021/acs.chemmater.1c02079
  • Y. Fang, H. P. Nair, L. Miao, B. Goodge, N. J. Schreiber, J. P. Ruf, L. F. Kourkoutis, K. M. Shen, D. G. Schlom, and B. J. Ramshaw
    Quantum oscillations and quasiparticle properties of thin film Sr2RuO4
    Physical Review B
    104
    (2021)
    10.1103/physrevb.104.045152
  • B. D. Faeth, S. Xie, S. Yang, J. K. Kawasaki, J. N. Nelson, S. Zhang, C. Parzyck, P. Mishra, C. Li, C. Jozwiak, A. Bostwick, E. Rotenberg, D. G. Schlom, and K. M. Shen
    Interfacial Electron-Phonon Coupling Constants Extracted from Intrinsic Replica Bands in Monolayer FeSe/SrTiO3
    Physical Review Letters
    127
    (2021)
    10.1103/physrevlett.127.016803
  • R. Jia, H. S. Kum, X. Sun, Y. Guo, B. Wang, P. Fang, J. Jiang, D. Gall, T. Lu, M. Washington, J. Kim, and J. Shi
    Van der Waals epitaxy and remote epitaxy of LiNbO3 thin films by pulsed laser deposition
    Journal of Vacuum Science & Technology A: Vacuum, Surfaces, and Films
    39
    (2021)
    10.1116/6.0001109
  • I. El Baggari, D. J. Baek, M. J. Zachman, D. Lu, Y. Hikita, H. Y. Hwang, E. A. Nowadnick, and L. F. Kourkoutis
    Charge order textures induced by non-linear couplings in a half-doped manganite
    Nature Communications
    12
    (2021)
    10.1038/s41467-021-24026-7
  • B.  . Faeth, S. -. Yang, J.  . Kawasaki, J.  . Nelson, P. Mishra, C.  . Parzyck, C. Li, D.  . Schlom, and K.  . Shen
    Incoherent Cooper Pairing and Pseudogap Behavior in Single-Layer FeSe/SrTiO3
    Physical Review X
    11
    (2021)
    10.1103/physrevx.11.021054
  • H. Kim, K. Lu, Y. Liu, H. S. Kum, K. S. Kim, K. Qiao, S. Bae, S. Lee, Y. J. Ji, K. H. Kim, H. Paik, S. Xie, H. Shin, C. Choi, J. H. Lee, C. Dong, J. A. Robinson, J. Lee, J. Ahn, G. Y. Yeom, D. G. Schlom, and J. Kim
    Impact of 2D–3D Heterointerface on Remote Epitaxial Interaction through Graphene
    ACS Nano
    15
    10587-10596
    (2021)
    10.1021/acsnano.1c03296
  • Z. Chen, Y. Jiang, Y. Shao, M. E. Holtz, M. Odstrčil, M. Guizar-Sicairos, I. Hanke, S. Ganschow, D. G. Schlom, and D. A. Muller
    Electron ptychography achieves atomic-resolution limits set by lattice vibrations
    Science
    372
    826-831
    (2021)
    10.1126/science.abg2533
  • P. B. Meisenheimer, R. A. Steinhardt, S. H. Sung, L. D. Williams, S. Zhuang, M. E. Nowakowski, S. Novakov, M. M. Torunbalci, B. Prasad, C. J. Zollner, Z. Wang, N. M. Dawley, J. Schubert, A. H. Hunter, S. Manipatruni, D. E. Nikonov, I. A. Young, L. Q. Chen, J. Bokor, S. A. Bhave, R. Ramesh, J. -. Hu, E. Kioupakis, R. Hovden, D. G. Schlom, and J. T. Heron
    Engineering new limits to magnetostriction through metastability in iron-gallium alloys
    Nature Communications
    12
    (2021)
    10.1038/s41467-021-22793-x
  • C. J. “. Wright, E. Dooryhée, L. A. Pressley, W. A. Phelan, P. G. Khalifah, and S. J. L. Billinge
    Toward In Situ Synchrotron Mapping of Crystal Selection Processes during Crystal Growth
    Chemistry of Materials
    33
    3359-3367
    (2021)
    10.1021/acs.chemmater.1c00602
  • Y. Guo, B. Goodge, L. Zhang, J. Jiang, Y. Chen, L. F. Kourkoutis, and J. Shi
    Unit-cell-thick domain in free-standing quasi-two-dimensional ferroelectric material
    Physical Review Materials
    5
    (2021)
    10.1103/physrevmaterials.5.044403
  • X. Zheng, E. Gerber, J. Park, D. Werder, O. Kigner, E. Kim, S. Xie, and D. G. Schlom
    Utilizing complex oxide substrates to control carrier concentration in large-area monolayer MoS2 films
    Applied Physics Letters
    118
    (2021)
    10.1063/5.0038383
  • J. P. Ruf, H. Paik, N. J. Schreiber, H. P. Nair, L. Miao, J. K. Kawasaki, J. N. Nelson, B. D. Faeth, Y. Lee, B. H. Goodge, B. Pamuk, C. J. Fennie, L. F. Kourkoutis, D. G. Schlom, and K. M. Shen
    Strain-stabilized superconductivity
    Nature Communications
    12
    (2021)
    10.1038/s41467-020-20252-7
  • M. R. Scudder, B. He, Y. Wang, A. Rai, D. G. Cahill, W. Windl, J. P. Heremans, and J. E. Goldberger
    Highly efficient transverse thermoelectric devices with Re4Si7 crystals
    Energy & Environmental Science
    14
    4009-4017
    (2021)
    10.1039/d1ee00923k
  • L. A. Pressley, A. Torrejon, W. A. Phelan, and T. M. McQueen
    Discovery and Single Crystal Growth of High Entropy Pyrochlores
    Inorganic Chemistry
    59
    17251-17258
    (2020)
    10.1021/acs.inorgchem.0c02479
  • A. Bhargava, R. Eppstein, J. Sun, M. A. Smeaton, H. Paik, L. F. Kourkoutis, D. G. Schlom, M. Caspary Toroker, and R. D. Robinson
    Breakdown of the Small‐Polaron Hopping Model in Higher‐Order Spinels
    Advanced Materials
    32
    (2020)
    10.1002/adma.202004490
  • I. El Baggari, N. Sivadas, G. M. Stiehl, J. Waelder, D. C. Ralph, C. J. Fennie, and L. F. Kourkoutis
    Direct Visualization of Trimerized States in 1T′−TaTe2
    Physical Review Letters
    125
    (2020)
    10.1103/physrevlett.125.165302
  • K. M. Adkison, S. Shang, B. J. Bocklund, D. Klimm, D. G. Schlom, and Z. Liu
    Suitability of binary oxides for molecular-beam epitaxy source materials: A comprehensive thermodynamic analysis
    APL Materials
    8
    (2020)
    10.1063/5.0013159
  • M. Straker, A. Chauhan, M. Sinha, W. A. Phelan, M. V. S. Chandrashekhar, K. J. Hemker, C. Marvel, and M. Spencer
    Growth of high purity zone-refined Boron Carbide single crystals by Laser Diode Floating Zone method
    Journal of Crystal Growth
    543
    125700
    (2020)
    10.1016/j.jcrysgro.2020.125700
  • Y. Ma, A. Edgeton, H. Paik, B. D. Faeth, C. T. Parzyck, B. Pamuk, S. Shang, Z. Liu, K. M. Shen, D. G. Schlom, and C. Eom
    Realization of Epitaxial Thin Films of the Topological Crystalline Insulator Sr3SnO
    Advanced Materials
    32
    (2020)
    10.1002/adma.202000809
  • K. A. DeRocher, P. J. M. Smeets, B. H. Goodge, M. J. Zachman, P. V. Balachandran, L. Stegbauer, M. J. Cohen, L. M. Gordon, J. M. Rondinelli, L. F. Kourkoutis, and D. Joester
    Chemical gradients in human enamel crystallites
    Nature
    583
    66-71
    (2020)
    10.1038/s41586-020-2433-3
  • Z. Chen, M. Odstrcil, Y. Jiang, Y. Han, M. Chiu, L. Li, and D. A. Muller
    Mixed-state electron ptychography enables sub-angstrom resolution imaging with picometer precision at low dose
    Nature Communications
    11
    (2020)
    10.1038/s41467-020-16688-6
  • B. H. Goodge, E. Bianco, N. Schnitzer, H. W. Zandbergen, and L. F. Kourkoutis
    Atomic-Resolution Cryo-STEM Across Continuously Variable Temperatures
    Microscopy and Microanalysis
    26
    439-446
    (2020)
    10.1017/s1431927620001427
  • A. B. Mei, I. Gray, Y. Tang, J. Schubert, D. Werder, J. Bartell, D. C. Ralph, G. D. Fuchs, and D. G. Schlom
    Local Photothermal Control of Phase Transitions for On‐Demand Room‐Temperature Rewritable Magnetic Patterning
    Advanced Materials
    32
    (2020)
    10.1002/adma.202001080
  • L. Miao, Y. Lee, A. B. Mei, M. J. Lawler, and K. M. Shen
    Two-dimensional magnetic monopole gas in an oxide heterostructure
    Nature Communications
    11
    (2020)
    10.1038/s41467-020-15213-z
  • E. Gerber, Y. Yao, T. A. Arias, and E. Kim
    Ab Initio Mismatched Interface Theory of Graphene on α−RuCl3 : Doping and Magnetism
    Physical Review Letters
    124
    (2020)
    10.1103/physrevlett.124.106804
  • H. S. Kum, H. Lee, S. Kim, S. Lindemann, W. Kong, K. Qiao, P. Chen, J. Irwin, J. H. Lee, S. Xie, S. Subramanian, J. Shim, S. Bae, C. Choi, L. Ranno, S. Seo, S. Lee, J. Bauer, H. Li, K. Lee, J. A. Robinson, C. A. Ross, D. G. Schlom, M. S. Rzchowski, C. Eom, and J. Kim
    Heterogeneous integration of single-crystalline complex-oxide membranes
    Nature
    578
    75-81
    (2020)
    10.1038/s41586-020-1939-z
  • M. Coll, J. Fontcuberta, M. Althammer, M. Bibes, H. Boschker, A. Calleja, G. Cheng, M. Cuoco, R. Dittmann, B. Dkhil, I. El Baggari, M. Fanciulli, I. Fina, E. Fortunato, C. Frontera, S. Fujita, V. Garcia, S. T. B. Goennenwein, C. -. Granqvist, J. Grollier, R. Gross, A. Hagfeldt, G. Herranz, K. Hono, E. Houwman, M. Huijben, A. Kalaboukhov, D. J. Keeble, G. Koster, L. F. Kourkoutis, J. Levy, M. Lira-Cantu, J. L. MacManus-Driscoll, J. Mannhart, R. Martins, S. Menzel, T. Mikolajick, M. Napari, M. D. Nguyen, G. Niklasson, C. Paillard, S. Panigrahi, G. Rijnders, F. Sánchez, P. Sanchis, S. Sanna, D. G. Schlom, U. Schroeder, K. M. Shen, A. Siemon, M. Spreitzer, H. Sukegawa, R. Tamayo, J. van den Brink, N. Pryds, and F. M. Granozio
    Towards Oxide Electronics: a Roadmap
    Applied Surface Science
    482
    1-93
    (2019)
    10.1016/j.apsusc.2019.03.312
  • H. Zheng, J. Zhang, B. Wang, D. Phelan, M. J. Krogstad, Y. Ren, W. A. Phelan, O. Chmaissem, B. Poudel, and J. F. Mitchell
    High pO2 Floating Zone Crystal Growth of the Perovskite Nickelate PrNiO3
    Crystals
    9
    324
    (2019)
    10.3390/cryst9070324
  • H. Boschker, T. Harada, T. Asaba, R. Ashoori, A.  . Boris, H. Hilgenkamp, C.  . Hughes, M.  . Holtz, L. Li, D.  . Muller, H. Nair, P. Reith, X. Renshaw Wang, D.  . Schlom, A. Soukiassian, and J. Mannhart
    Ferromagnetism and Conductivity in Atomically Thin SrRuO3
    Physical Review X
    9
    (2019)
    10.1103/physrevx.9.011027
  • B. H. Savitzky, I. El Baggari, C. B. Clement, E. Waite, B. H. Goodge, D. J. Baek, J. P. Sheckelton, C. Pasco, H. Nair, N. J. Schreiber, J. Hoffman, A. S. Admasu, J. Kim, S. Cheong, A. Bhattacharya, D. G. Schlom, T. M. McQueen, R. Hovden, and L. F. Kourkoutis
    Image registration of low signal-to-noise cryo-STEM data
    Ultramicroscopy
    191
    56-65
    (2018)
    10.1016/j.ultramic.2018.04.008
  • K. Kang, K. Lee, Y. Han, H. Gao, S. Xie, D. A. Muller, and J. Park
    Layer-by-layer assembly of two-dimensional materials into wafer-scale heterostructures
    Nature
    550
    229-233
    (2017)
    10.1038/nature23905
  • Y. Hsu, A. Vaezi, M. H. Fischer, and E. Kim
    Topological superconductivity in monolayer transition metal dichalcogenides
    Nature Communications
    8
    (2017)
    10.1038/ncomms14985
  • D. MacNeill, G. M. Stiehl, M. H. D. Guimaraes, R. A. Buhrman, J. Park, and D. C. Ralph
    Control of spin–orbit torques through crystal symmetry in WTe2/ferromagnet bilayers
    Nature Physics
    13
    300-305
    (2016)
    10.1038/nphys3933
View All Publications
People
  • Darrell Schlom
    Synthesis
  • Tyrel McQueen
    Director of Bulk Crystal Facility Chemistry
    Chemistry
  • Thomas Dienel
    Director of User Program
    Materials Science & Engineering
  • David A. Muller
    Director of Electron Microscopy Facility
    Applied & Engineering Physics
  • Tomás Arias
    Director of Theory User Facility Physics
    Physics
  • Jie Shan
    Director of Thin Film Facility
    Applied & Engineering Physics
View All People
Universities
CONTACT:

National Science Foundation

Division of Materials Research

2415 Eisenhower Avenue

Alexandria, VA 22314

Any opinions, findings and conclusions or recommendations expressed in this material are those of the author(s) and do not necessarily reflect the views of the National Science Foundation.